Abstract
We investigate direct above-threshold ionization in diatomic molecules, with\nparticular emphasis on how quantum interference is altered by a driving field\nof non-vanishing ellipticity. This interference may be either temporal, i.e.,\nrelated to ionization events occurring at different times, or spatial, i.e.,\nrelated to the electron emission at different centers in the molecule.\nEmploying the strong-field approximation and saddle-point methods, we find\nthat, in general, for non-vanishing ellipticity, there will be a blurring of\nthe temporal and spatial interference patterns. The former blurring is caused\nby the electron velocity component perpendicular to the major polarization\naxis, while spatial interference is washed out as a consequence either of s-p\nmixing, or of the temporal dependence of the ionization prefactor. Both types\nof interference are analyzed in detail in terms of electron trajectories, and\nspecific conditions for which sharp fringes occur are provided.\n
Keywords
Affiliated Institutions
Related Publications
High-order-harmonic generation from diatomic molecules in driving fields with nonvanishing ellipticity: A generalized interference condition
We investigate the influence of intense, elliptically polarized driving fields on high-order harmonic spectra from aligned diatomic molecules. We derive a generalized two-center...
Plasma perspective on strong field multiphoton ionization
During strong-field multiphoton ionization, a wave packet is formed each time the laser field passes its maximum value. Within the first laser period after ionization there is a...
Signatures of Molecular Orbital Structure in Lateral Electron Momentum Distributions from Strong-Field Ionization
Strong-field ionization of aligned diatomic and polyatomic molecules such as O2, N2, C2H4, and others in circularly polarized laser fields is investigated theoretically. By calc...
Publication Info
- Year
- 2013
- Type
- article
- Volume
- 88
- Issue
- 1
- Citations
- 22
- Access
- Closed
External Links
Social Impact
Social media, news, blog, policy document mentions
Citation Metrics
Cite This
Identifiers
- DOI
- 10.1103/physreva.88.013406