Abstract

The electronic structure of p-type doped Bi2Te3 is studied by angle-resolved photoemission spectroscopy (ARPES) to experimentally confirm the mechanism responsible for the high thermoelectric figure of merit. Our ARPES study shows that the band edges are located off. the Gamma-Z line in the Brillouin zone, which provides direct observation that the spin-orbit interaction is a key factor to understand the electronic structure and the corresponding thermoelectric properties of Bi2Te3. A successive time-dependent ARPES measurement also reveals that the electron-like bands crossing E-F near the (Gamma) under bar -point are formed in an hour after cleaving the crystals. We interpret these as surface states induced by surface band bending, possibly due to quintuple inter-layer distance change of Bi2Te3. Copyright (c) EPLA, 2008.

Keywords

Angle-resolved photoemission spectroscopyBrillouin zonePhotoemission spectroscopyCondensed matter physicsElectronic structureElectronic band structureBand bendingX-ray photoelectron spectroscopySpin–orbit interactionMaterials scienceSpin (aerodynamics)Thermoelectric effectSpectroscopyPhysicsNuclear magnetic resonanceQuantum mechanics

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Publication Info

Year
2008
Type
article
Volume
81
Issue
5
Pages
57006-57006
Citations
108
Access
Closed

Citation Metrics

108
OpenAlex
4
Influential
99
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Cite This

H.‐J. Noh, H. Koh, S.-J. Oh et al. (2008). Spin-orbit interaction effect in the electronic structure of Bi <sub>2</sub> Te <sub>3</sub> observed by angle-resolved photoemission spectroscopy. Europhysics Letters (EPL) , 81 (5) , 57006-57006. https://doi.org/10.1209/0295-5075/81/57006

Identifiers

DOI
10.1209/0295-5075/81/57006
arXiv
0803.0052

Data Quality

Data completeness: 84%