Abstract

This paper describes an instrument capable of studying diffuse reflection of mid-infrared (mid-IR) photons on ultrafast time scales. Femtosecond mid-IR pulses are generated by difference frequency mixing the output of an optical parametric amplifier that is pumped using a regeneratively amplified Ti:Sapphire laser. Time resolution is achieved by up-converting the diffusely reflected photons with pulses from the Ti:Sapphire oscillator. Experiments were performed on a series of powdered KBr samples containing varying amounts of carbon black. The results suggest that diffusely reflected mid-IR photons fall into two distinct categories. A small fraction of the photons travel relatively long effective path lengths (1.3–2.3 mm), while the majority traverse a much shorter distance (0.2–0.05 mm).

Keywords

InfraredUltrashort pulseDiffuse reflectionReflection (computer programming)OpticsDiffuse reflectance infrared fourier transformMaterials scienceChemistryPhysicsComputer scienceLaser

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Publication Info

Year
2014
Type
article
Volume
68
Issue
1
Pages
1-4
Citations
7
Access
Closed

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Eric B. Brauns (2014). Mid-Infrared Diffuse Reflection on Ultrafast Time Scales. Applied Spectroscopy , 68 (1) , 1-4. https://doi.org/10.1366/13-07258

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DOI
10.1366/13-07258