Abstract

The electrochemical reduction of carbon dioxide (CO<sub>2</sub>) has received significant attention in academic research, although the techno-economic prospects of the technology for the large-scale production of chemicals are unclear. In this work, we briefly reviewed the current state-of-the-art CO<sub>2</sub> reduction figures of merit, and performed an economic analysis of a generalized CO<sub>2</sub> electrolyzer system for the production of 100 tons/day of various CO<sub>2</sub> reduction products. While carbon monoxide and formic acid were the most economically favorable products under current conditions, higher-order alcohols such as ethanol and n-propanol could be highly promising if reasonable electrocatalytic performance benchmarks were achieved. Furthermore, we established performance targets such that if these targets are achieved, electrochemical CO<sub>2</sub> reduction for fuels and chemicals production can become a profitable option as part of the growing renewable energy infrastructure.

Keywords

OverpotentialElectrolysisEnvironmental scienceRenewable energyProduction (economics)Electrochemical reduction of carbon dioxideNet present valueCarbon monoxideProcess engineeringWaste managementPulp and paper industryElectrochemistryChemistryEconomicsEngineeringCatalysis

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Publication Info

Year
2018
Type
article
Volume
57
Issue
6
Pages
2165-2177
Citations
1391
Access
Closed

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Cite This

Matthew Jouny, Wesley Luc, Feng Jiao (2018). General Techno-Economic Analysis of CO<sub>2</sub> Electrolysis Systems. Industrial & Engineering Chemistry Research , 57 (6) , 2165-2177. https://doi.org/10.1021/acs.iecr.7b03514

Identifiers

DOI
10.1021/acs.iecr.7b03514